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Dual-Wavelength Spectrum-Shaped Mid-Infrared Pulses and Steering High-Harmonic Generation in Solids
- Ultrafast Science Vol. 3, Issue 3, (2023)
- Affiliations：
a College of Electronics and Information Engineering, Sichuan University, Chengdu, Sichuan 610064, China. b Key Laboratory of High Energy Density Physics and Technology (MoE), College of Physics, Sichuan University, Chengdu 610064, China.c College of Physics, Key Laboratory of High Energy Density Physics and Technology of the Ministry of Education, Sichuan University,Sichuan,Chengdu,China,610064
- Author bio：
- Funds：
DOI：10.34133/ultrafastscience.0022
CLC：Published：2023，
- Accepted：
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Linzhen He, Weizhe Wang, Kan Tian, Maoxing Xiang, Zhongjun Wan, Bo Hu, Yang Li, Han Wu, Zi-Yu Chen, Fan Yang, Houkun Liang. 2023: Dual-Wavelength Spectrum-Shaped Mid-Infrared Pulses and Steering High-Harmonic Generation in Solids. 超快科学, 3(3).
Linzhen He, Weizhe Wang, Kan Tian, Maoxing Xiang, Zhongjun Wan, Bo Hu, Yang Li, Han Wu, Zi-Yu Chen, Fan Yang, Houkun Liang. 2023: Dual-Wavelength Spectrum-Shaped Mid-Infrared Pulses and Steering High-Harmonic Generation in Solids. Ultrafast Science, 3(3).
Linzhen He, Weizhe Wang, Kan Tian, Maoxing Xiang, Zhongjun Wan, Bo Hu, Yang Li, Han Wu, Zi-Yu Chen, Fan Yang, Houkun Liang. 2023: Dual-Wavelength Spectrum-Shaped Mid-Infrared Pulses and Steering High-Harmonic Generation in Solids. 超快科学, 3(3). DOI： 10.34133/ultrafastscience.0022
Linzhen He, Weizhe Wang, Kan Tian, Maoxing Xiang, Zhongjun Wan, Bo Hu, Yang Li, Han Wu, Zi-Yu Chen, Fan Yang, Houkun Liang. 2023: Dual-Wavelength Spectrum-Shaped Mid-Infrared Pulses and Steering High-Harmonic Generation in Solids. Ultrafast Science, 3(3). DOI： 10.34133/ultrafastscience.0022
摘要
Mid-infrared (MIR) ultra-short pulses with multiple spectral-band coverage and good freedom in spectral and temporal shaping are desired by broad applications such as steering strong-field ionization
investigating bound-electron dynamics
and minimally invasive tissue ablation. However
the existing methods of light transient generation lack freedom in spectral tuning and require sophisticated apparatus for complicated phase and noise control. Here
with both numerical analysis and experimental demonstration
we report the first attempt
to the best our knowledge
at generating MIR pulses with dualwavelength spectral shaping and exceptional freedom of tunability in both the lasing wavelength and relative spectral amplitudes
based on a relatively simple and compact apparatus compared to traditional pulse synthesizers. The proof-of-concept demonstration in steering the high-harmonic generation in a polycrystalline ZnSe plate is facilitated by dual-wavelength MIR pulses shaped in both spectral and temporal domains
spanning from 5.6 to 11.4 μm
with multi-microjoule pulse energy and hundred- milliwatt average power. Multisets of harmonics corresponding to different fundamental wavelengths are simultaneously generated in the deep ultraviolet region
and both the relative strength of individual harmonics sets and the spectral shapes of harmonics are harnessed with remarkable freedom and flexibility. This work would open new possibilities in exploring femtosecond control of electron dynamics and light–matter interaction in composite molecular systems.
Abstract
Mid-infrared (MIR) ultra-short pulses with multiple spectral-band coverage and good freedom in spectral and temporal shaping are desired by broad applications such as steering strong-field ionization
investigating bound-electron dynamics
and minimally invasive tissue ablation. However
the existing methods of light transient generation lack freedom in spectral tuning and require sophisticated apparatus for complicated phase and noise control. Here
with both numerical analysis and experimental demonstration
we report the first attempt
to the best our knowledge
at generating MIR pulses with dualwavelength spectral shaping and exceptional freedom of tunability in both the lasing wavelength and relative spectral amplitudes
based on a relatively simple and compact apparatus compared to traditional pulse synthesizers. The proof-of-concept demonstration in steering the high-harmonic generation in a polycrystalline ZnSe plate is facilitated by dual-wavelength MIR pulses shaped in both spectral and temporal domains
spanning from 5.6 to 11.4 μm
with multi-microjoule pulse energy and hundred- milliwatt average power. Multisets of harmonics corresponding to different fundamental wavelengths are simultaneously generated in the deep ultraviolet region
and both the relative strength of individual harmonics sets and the spectral shapes of harmonics are harnessed with remarkable freedom and flexibility. This work would open new possibilities in exploring femtosecond control of electron dynamics and light–matter interaction in composite molecular systems.
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references
He, L., Wu, H., Wang, W. et al. Long-wavelength infrared upconversion time-stretch spectroscopy. Applied Physics Letters, 2024, 125(7): 071102. DOI:10.1063/5.0218110.
He, L., Wu, H., Wang, W. et al. Long-wavelength infrared upconversion time-stretch spectroscopy. Applied Physics Letters, 2024, 125(7): 071102. DOI:10.1063/5.0218110.
Tian, K., Xiang, M., Wen, X. et al. Tissue Ablation with Multi-Millimeter Depth and Cellular-Scale Collateral Damage by a Femtosecond Mid-Infrared Laser Tuned to the Amide-I Vibration. Laser and Photonics Reviews, 2024, 18(2): 2300421. DOI:10.1002/lpor.202300421.
Tian, K., Xiang, M., Wen, X. et al. Tissue Ablation with Multi-Millimeter Depth and Cellular-Scale Collateral Damage by a Femtosecond Mid-Infrared Laser Tuned to the Amide-I Vibration. Laser and Photonics Reviews, 2024, 18(2): 2300421. DOI:10.1002/lpor.202300421.
Boukhaoui, D., Idlahcen, S., Houard, J. et al. High harmonic generation in Solids driven by high energy fiber laser source. Proceedings of SPIE - The International Society for Optical Engineering, 2024. DOI:10.1117/12.3022412.
Boukhaoui, D., Idlahcen, S., Houard, J. et al. High harmonic generation in Solids driven by high energy fiber laser source. Proceedings of SPIE - The International Society for Optical Engineering, 2024. DOI:10.1117/12.3022412.
Long, Z., Yang, H., Tian, K. et al. High-harmonic generation in CdTe with ultra-low pump intensity and high photon flux. Communications Physics, 2023, 6(1): 228. DOI:10.1038/s42005-023-01354-2.
Long, Z., Yang, H., Tian, K. et al. High-harmonic generation in CdTe with ultra-low pump intensity and high photon flux. Communications Physics, 2023, 6(1): 228. DOI:10.1038/s42005-023-01354-2.
Wan, Z., Guan, Z., Liu, J. et al. Wavelength scaling of high harmonic yields and cutoff energies in solids driven by mid-infrared pulses. Optics Express, 2023, 31(19): 30294-30304. DOI:10.1364/OE.497641.
Wan, Z., Guan, Z., Liu, J. et al. Wavelength scaling of high harmonic yields and cutoff energies in solids driven by mid-infrared pulses. Optics Express, 2023, 31(19): 30294-30304. DOI:10.1364/OE.497641.
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